Near-field intensity correlations in semicontinuous metal-dielectric films.
نویسندگان
چکیده
Spatial intensity correlation functions are obtained from near-field scanning optical microscope measurements of semicontinuous metal-dielectric films. The concentration of metal particles on a dielectric surface is varied over a wide range to control the scattering strength. At low and high metal coverages where scattering is weak, the intensity correlation functions exhibit oscillations in the direction of incident light due to excitation of propagating surface waves. In the intermediate regime of metal concentration, the oscillatory behavior is replaced by a monotonic decay as a result of strong scattering and anomalous absorption. Significant differences in the near-field intensity correlations between metallic and dielectric random systems are demonstrated.
منابع مشابه
Surface plasmon delocalization by short-range correlations in percolating metal systems
Theoretical and experimental studies of the electromagnetic response of semicontinuous metal films are presented. A scaling theory is developed by solving the surface plasmon eigenproblem. The short-range correlations in the governing Kirchhoff Hamiltonian result in delocalization of the surface plasmon eigenmodes. Although their relative weight in the spectrum becomes asymptotically small for ...
متن کاملGrowth, morphology, and optical and electrical properties of semicontinuous metallic films
The growth and optical properties of semicontinuous silver films on insulator substrates were studied experimentally and theoretically. In the experimental studies, films were synthesized by the pulsed-laser deposition technique, characterized by electron microscopy and in situ optical and dc electrical resistance measurements and studied using near-field optical microscopy. The percolation thr...
متن کاملCoexistence of localized and delocalized surface plasmon modes in percolating metal films.
Near-field intensity statistics in semicontinuous silver films over a wide range of surface coverage are investigated using near-field scanning optical microscopy. The variance of intensity fluctuations and the high-order moments of intensity enhancement exhibit local minima at the percolation threshold. This reduction in local field fluctuations results from resonant excitation of delocalized ...
متن کاملSurface plasmon excitation and correlation-induced localization-delocalization transition in semicontinuous metal films
By solving the surface plasmon SP eigenproblem, a scaling theory is developed for the electromagnetic response of semicontinuous metal films. It is shown that short-range correlations in the governing Kirchhoff Hamiltonian result in delocalization of the SP eigenmodes in the center of the spectrum. The subset of those modes has a zero measure so that their relative weight in the spectrum become...
متن کاملNonlinear optics of random metal-dielectric films
Surface-enhanced optical nonlinearities are studied in a semicontinuous film consisting of metal granules randomly distributed on an insulating substrate. The local fields are very inhomogeneous in such films and consist of strongly localized sharp peaks. In peaks ~‘‘hot’’ spots!, the local fields exceed the applied field by several orders of magnitudes resulting in giant enhancements of the op...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
عنوان ژورنال:
- Physical review letters
دوره 94 22 شماره
صفحات -
تاریخ انتشار 2005